Progress of SAFERIB: General Aspects - WP5

52,54Mn, 52,59Fe, 55,56,57,58,60Co, 57Ni, 62,65Zn, 67Ga. 238U – Cu (nat). 7Be, 22 ... radioactivity of transport lines and post-accelerator. - radioactivity in ...
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Progress of SAFERIB: General Aspects P.G. Thirolf, LMU München

Part of the EURONS Integrated Infrastructure Initiative - Radiation Protection Issues related to Radioactive Ion Beam Facilities (LMU, CERN, FZJ, GANIL, GSI, INFN-LNL)

News from EURONS coordinator: • 1st annual report has not yet been approved by EC, due to modifications requested around Transnational Access to Large Scale Infrastructures -> prefinancing of EURONS (and SAFERIB) on the level of still available reserve at management team.

Peter Thirolf, JRA-10 SAFERIB

EURISOL-DS (T5)/SAFERIB Progress Meeting, Munich, October 12./13., 2006

Project Tasks

Task T-J10-1: Radiation-correlated mechanical, thermal, electric material properties Subtask T-J10-1.1: Characterization of hot open fission source (LMU) Subtask T-J10-1.2: Secondary radiation and activation by fast heavy-ion beams in thick targets (GSI) Task T-J10-2: Migration of radioactivity Subtask T-J10-2.1: Reliability of codes (CERN) Subtask T-J10-2.2: Release study (CERN) (FZJ) Subtask T-J10-2.3: Soil/ground water activation Subtask T-J10-2.4: Technical concept to confine radioactivity (GANIL) Task T-J10-3: Technical concept to confine volatile radioactivity (GANIL) Task T-J10-4: Failsafe remote-controlled target manipulator

Peter Thirolf, JRA-10 SAFERIB

(INFN-LNL)

EURISOL-DS (T5)/SAFERIB Progress Meeting, Munich, October 12./13., 2006

Status of Milestones, Deliverables Milestones:

Short title

M-J10-1.1

Properties of fission source prototype characterized Secondary radiation from thick targets Activation measurements and activation Calculations of components in the vicinity of thick In-flight targets Validation of reliability: isotope production codes Release study of radiologically important isotopes from target ion source Study of soil/ground water activation Concept to confine radioactivity Technical concept to confine volatile radioactivity Solution for radiation-hard , remote-controlled target manipulator

M-J10-1.2 M-J10-1.3

M-J10-2.1 M-J10-2.2 M-J10-2.3 M-J10-2.4 M-J10-3 M-J10-4

Date duei 12/06

Date accompl.

12/05 12/07

12/05

12/05 4/06

10/05 04/06

6/06 6/06 11/07 11/07

11/06 ? 10/06 ?

Short title

Date due

D-J10-1

Report on task T-J10-1 (material properties) Report on task T-J10-2 (migration of activity) Report on task T-J10-3 (containment of volatile activity) Report on task T-J10-4 ( remote-controlled manipulator)

12/07

Type Disseminati on level R/PU

12/07

R/PU

12/07

R/PU

12/07

R/PU

D-J10-3 D-J10-4

Peter Thirolf, JRA-10 SAFERIB

LMU GSI

*

GSI

Deliverables

D-J10-2

Remark

Date delivered

CERN CERN FZJ GANIL GANIL INFN

( ) ( )

Remark

EURISOL-DS (T5)/SAFERIB Progress Meeting, Munich, October 12./13., 2006

LMU progress for SAFERIB 06/06 - 10/06 Task: Characterization of fission source prototype: heating tests beam emittance

Peter Thirolf, JRA-10 SAFERIB

EURISOL-DS (T5)/SAFERIB Progress Meeting, Munich, October 12./13., 2006

LMU progress for SAFERIB 06/06 - 10/06 Nd mass spectrum from source prototype: 142 144

beam emittance: 146

y Integral: 10,5π mm mrad @ 21 keV 0

Here: 143 emittance plot !!

10

2,5E-13 5E-13

145 148 150

1E-12 1,25E-12 1,5E-12

b [mrad]

133Cs

7,5E-13

5

1,75E-12

0

2E-12

-5

intensities according to isotopic abundances

-10 0

5

10

15

y [mm]

10.5 π mm mrad (@ 21 keV) Peter Thirolf, JRA-10 SAFERIB

EURISOL-DS (T5)/SAFERIB Progress Meeting, Munich, October 12./13., 2006

LMU progress for SAFERIB 06/06 - 10/06 Thermal effects: tilt of Re cylinder support

C-sublimation onto insulators Peter Thirolf, JRA-10 SAFERIB

EURISOL-DS (T5)/SAFERIB Progress Meeting, Munich, October 12./13., 2006

GSI activities for SAFERIB 06/06 - 10/06 G. Fehrenbacher, E. Kozlova, A. Knapp, T. Radon (GSI, department for safety and radiation protection)

Task: Activation of components in the vicinity of thick in-flight targets Activation experiments in Cave A final goal: induced activity per radionuclide in components beam parameters: U-238 on stack of Cu and steel disks @ 120 MeV/u and 500 MeV/u Comparison with MC-Code FLUKA 2005.6

Peter Thirolf, JRA-10 SAFERIB

EURISOL-DS (T5)/SAFERIB Progress Meeting, Munich, October 12./13., 2006

Targets for the Uranium beam irradiation

Al 100 µm 238U

beam Vacuum

600 mm

Material and configuration

Initial energy of 238U ions

Target thickness

Irradiation time, h / Total dose on the target (ions)

1

Stainless steel 302 – set of disks mm: 0.1, 0.5, 0.5

120 MeV/u

1.1 mm

6.3 / 2.01*1011

2

Cu – set of 11 disks of 0.1 mm

120 MeV/u

1.1 mm

12.25 / 3.32*1011

3

Stainless steel 302 – set of 35 disks

500 MeV/u

11.9 mm

16.35 / 2.352*1011

4

Cu – set of 34 disks

500 MeV/u

11 mm

20.0 / 4.66*1011

Target N

Air

SEETRAM (beam monitor)

The 0.1 – millimeter foils were inserted after each thick disk, which allowed to obtain the spatial distribution of the activation rates in the target along the range Peter Thirolf, JRA-10 SAFERIB

EURISOL-DS (T5)/SAFERIB Progress Meeting, Munich, October 12./13., 2006

Residual Nuclides Measured in Copper and Stainless Steel Targets

Projectile – activation target 238U

Residual nuclides in activation target 7Be, 22,24Na, 28Mg, 41Ar, 42,43K, 44,44M,46,47,48Sc,

– Stainless steel

48V, 48,51Cr, 52,54,56Mn, 52,59Fe, 55,56,57,58Co, 56,57Ni 7Be, 22,24Na, 28Mg, 42,43K, 44,44M,46,47,48Sc, 48V,

238U

48,51Cr,

– Cu (nat)

52,54Mn, 52,59Fe, 55,56,57,58,60Co, 57Ni, 62,65Zn, 67Ga

Distribution of activity in the copper target after Residual activity, (Bq/p.p.)

1.00E-08

238

U 500 Mev/u irradiation

2.25

9.00E-09

Experiment

8.00E-09

1.37

FLUKA

7.00E-09 6.00E-09 5.00E-09 4.00E-09 3.00E-09 2.00E-09 1.00E-09

Ratio: 3.19

1.54

1.59

Co-56

Co-57

1.40

Some of the projectile fragments, which are observed in activation copper and stainless steel foils: 127Xe, 237U, 140Ba, 206Bi, 131Ba, 103Ru, 88Y, 99Mo

0.00E+00 Sc-46

Peter Thirolf, JRA-10 SAFERIB

Cr-51

Mn-54

Co-58

EURISOL-DS (T5)/SAFERIB Progress Meeting, Munich, October 12./13., 2006

GANIL progress report: SAFERIB Manssour FADIL , Bertrand RANNOU Tasks: scientific and technical studies (SAFERIB): expansion of contamination and migration of radioactive gases: - radioactivity of transport lines and post-accelerator - radioactivity in experimental areas radioactive gases storage legal study (EURISOL): conformity to legislation Peter Thirolf, JRA-10 SAFERIB

EURISOL-DS (T5)/SAFERIB Progress Meeting, Munich, October 12./13., 2006

Expansion of contamination and migration of radioactive gases: Concept and design studies of the cryotraps: Concept and design studies of the cryogenic source (collaboration with IPN/Orsay):

done in 2005

finished in October 2006

Beginning of the construction (cryotraps and source):

November 2006

First experimental tests (cryotraps and source)

March 2007

deliverable: technical report (design and experimental tests) Peter Thirolf, JRA-10 SAFERIB

EURISOL-DS (T5)/SAFERIB Progress Meeting, Munich, October 12./13., 2006

Radioactive gases storage: Conception studies (Collaboration with industrial company ): done in September 2006 improvements to be brought deliverable: detailed technical report

Peter Thirolf, JRA-10 SAFERIB

EURISOL-DS (T5)/SAFERIB Progress Meeting, Munich, October 12./13., 2006

Forschungszentrum Jülich in der Helmholtz-Gemeinschaft

FZJ: Activity migration in ground water • Work on coupling TRACE/PARTRACE (code for transport calculations of nuclides in groundwater) with the water/soil activation module was started; improved results are expected for September ’06 • The literature survey on KD-values is almost complete • Calculations on activation profiles in CERN-type soil around a 10 MW/1.334 GeV LINAC were documented and a respective draft report is available -> talks by R. Moormann and N. Prolingheuer Institut für Sicherheitsforschung und Reaktortechnik - ISR Peter Thirolf, JRA-10 SAFERIB

Rainer Moormann

EURISOL-DS (T5)/SAFERIB Progress Meeting, Munich, October 12./13., 2006

SPES concept for target removal

extension to EURISOL

Design considerations: o efficient target handling/servicing system for frequent, quick changes o target area: high residual activity, contamination with mobile activity o target maintenance: remote disconnecting/transfer to hot cell o manipulator system for all actions in hot cell needed o requirements: dissassembling/reassembling of all target components o manipulator fitted with cutting and welding tools Peter Thirolf, JRA-10 SAFERIB

EURISOL-DS (T5)/SAFERIB Progress Meeting, Munich, October 12./13., 2006

Peter Thirolf, JRA-10 SAFERIB

EURISOL-DS (T5)/SAFERIB Progress Meeting, Munich, October 12./13., 2006

Peter Thirolf, JRA-10 SAFERIB

EURISOL-DS (T5)/SAFERIB Progress Meeting, Munich, October 12./13., 2006

Peter Thirolf, JRA-10 SAFERIB

EURISOL-DS (T5)/SAFERIB Progress Meeting, Munich, October 12./13., 2006

Peter Thirolf, JRA-10 SAFERIB

EURISOL-DS (T5)/SAFERIB Progress Meeting, Munich, October 12./13., 2006