Task 5 “Safety & Radioprotection” - WP5

Oct 28, 2005 - 9-months Progress Report. NIPNE-Bucharest (Romania) ... -PEANUT event generator(hadron-nucleus interactions). -RQMD & DPMJET-II ...
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EURISOL-DS / Task 5 “Safety & Radioprotection” 9-months Progress Report NIPNE-Bucharest (Romania) 1 Sub-Task A: Radiation, activation, shielding & doses • Neutron attenuation calculations: comparison with data Simulations with FLUKA: - HIMAC benchmarck - basic shielding studies (see next presentation)

1 Sub-Task B: Radioactivity control, safety and risks • Dispersion of radio-elements, contamination, migration: experience gained from NPPs (D. Vamanu, B. Vamanu, V. Acasandrei) Development of an integrated software platform: “Safety and Radioprotection Desktop Toolkit” and of an e-book (see presentation of B.Vamanu) Period Pers. (k€ ) Consum.(k€ ) Travel (k€ ) Total (k€ ) FTE Contr./Total (man*years) 9 months (actual) 2.8 0 1.2 4.0 0.3 / 0.8 1st year (estimation) 4.2 0 1.2 5.4 0.5 / 1.2 2nd year (request) 8.4 0 2.5 10.9 1.0 / 2.5 4 years (approuved) 16.6 3.3 8.4 28.3 2.0 / 8.0 CEA-Saclay, 27-28 October, 2005

F. Negoita, [email protected]

EURISOL+SAFERIB Meeting CEA-Saclay, 27-28 October 2005

High energy neutron 1 attenuation studies 1

1

-status of the work-

INTRODUCTION 1 1

1 1 1

Goal: to develop a calculation strategy for a M onte Carlo simulation of EURI SOL Facility radiation protection design; FLUKA M onte Carlo calculations focused on high energy neutron behavior: - energy dependence of neutron radiation fields i - resulting ambient dose equivalent distributions; Computer simulations use simple geometry, different wall thicknesses; Two homogeneous bulk-shielding materials: iron and concrete are investigated; A comparison between the result s of the FLUKA code to data from the current literature is provided.

EURISOL Meeting, CEA Saclay, 27-28 October 2005

Modelling approach (1) 1 • •

1 •

1 • •

Source neutron Monoenergetic (1 GeV ) neutron transmission Attenuation of secondary neutrons produced by: - high energy protons - 12C heavy ions on Cu target (HIMAC- benchmarck experiment)

Geometry Plane of 4m (iron) and 5 m (concrete) thick with normal incident parallel beams

Shielding Material Iron (Density 7.87 g/cm3) Concrete (Density 2.27 g/cm3) [Type 02-a, ANL-5800, 660(1963)]

EURISOL Meeting, CEA Saclay, 27-28 October 2005

Modelling approach (2) 1

• •



Calculated quantities Neutron spectrum whole energy range but thermal group (0.414eV) Dose equivalent due to the neutrons; - Above 20 MeV (M. Pelliccioni at al, RPD 88, pp. 279, (2000)), fluence to ambient dose conversion coefficients Attenuation lengths in iron and concrete obtained by MINUIT/PAW fitting subroutine

EURISOL Meeting, CEA Saclay, 27-28 October 2005

Monte Carlo simulations Parameter settings FLUKA– interaction and transport code 1

1

1

Physical models* -PEANUT event generator (hadron-nucleus interactions) -RQMD & DPMJET-II external event generator (nucleus-nucleus interaction) Transport cut-off energy set at 0.414eV or 19.6MeV for high energy account Low-energy neutron cross section library (72 groups) used below19.6MeV

Biasing - Russian rullete and splitting at boundary crossing based on region relative importance - Region-dependent weight window in three energy ranges

* Fasso, A, Ferrari, A, Ranft, J, Sala P.R. Status and Proscpective for Hadronic Applications, Proceeding of the Monte Carlo 2000 Conference, Lisbone October 2000, Springler -Verlag Berlin EURISOL Meeting, CEA Saclay, 27-28 October 2005

Deep penetration Characteristics 1GeV proton on Pb target model*

CONCRETE shield 5m concrete slab

1

high energy tail major component of the spectra;

1

the intermediate energy spectra are closed to 1/E distribution;

1

Energy spectra of neutrons at various concrete depths 1.0E+0 1.0E-1

in the low energy region concrete has a high shielding performance due to elastic scattering effect of hydrogen;

E* dF/dE (cm^-2 pr^-1)



1.0E-2 1.0E-3 1.0E-4 1.0E-5 1.0E-6

100cm 200cm

1.0E-7 1.0E-8

300cm 400cm 500cm

1.0E-9 1.0E-9

1.0E-7

1.0E-5

1.0E-3

Energy (GeV) *

Baseline parameters from Eurisol-DS #3 “100kW direct target station” EURISOL Meeting, CEA Saclay, 27-28 October 2005

1.0E-1

Deep penetration Characteristics 1GeV proton on Pb target model*

IRON shield •

Energy spectra of neutrons at various iron depths

4m iron slab

1.0E+0

300 cm

1 1

1

typical equilibrium spectra with a shape which is independent of the shield thickness; attenuation of the neutron spectrum with increasing shield thickness; major energy component shifts towards the low energy range due to elastic scattering and 24 keV iron resonance;

E*dF/dE (cm^-2 pr^-)1

1.0E-1

1

100 cm 200 cm

1.0E-2 1.0E-3 1.0E-4 1.0E-5 1.0E-6 1.0E-7 1.0E-8 1.0E-10

low energy neutron flux (E< hundreds of keV) attenuates slower than high energy tail being build-up from the inelastic scattering of high energy neutrons

1.0E-8

1.0E-6

1.0E-4

1.0E-2

Energy (GeV)

* Baseline parameters from Eurisol-DS #3 “100kW direct target station” EURISOL Meeting, CEA Saclay, 27-28 October 2005

1.0E+0

Deep penetration Characteristics 1GeV proton on Pb target model*

DOUBLED-LAYERED shield , case 1 1 1 1

(1m Iron + 4m Concrete) slab

Neutron energy spectra four a double- layered shield, case 1 1.0E+1

50cm 100 cm 200 cm 300 cm

high energy neutron tail is the major component in the outer layer of the shield; influence of concrete component in absorbing low energy neutron the shield performance for a source strength of 6.242E+14 p/s (corresponding to I=1001A) has to be improved

E * dF/dE (cm^-2 pr^-1)



1.0E+0

400 cm

1.0E-1

500cm

1.0E-2 1.0E-3 1.0E-4 1.0E-5 1.0E-6 1.0E-7 1.0E-8 1.0E-101.0E-9 1.0E-8 1.0E-7 1.0E-6 1.0E-5 1.0E-4 1.0E-3 1.0E-2 1.0E-1 1.0E+0

Energy (Gev)

* Baseline parameters from Eurisol-DS #3 “100kW direct target station” EURISOL Meeting, CEA Saclay, 27-28 October 2005

Deep penetration Characteristics 1GeV proton on Pb target model*

DOUBLED-LAYERED shield , case 2 Neutron energy spectra for a double-layer shield, case 2

1

neutron flux is dominated by the contribution of the low energy neutron in the outer iron layer;

1

The low energy flux is reduced quite effectively by the concrete layer;

1

shielding potential of this double layered shield w.r.t. case 1

Fluence (cm^-2 pr-1)

(4m Iron + 1m Concrete) slab



1.0E+0 1.0E-1 1.0E-2 1.0E-3 1.0E-4 1.0E-5 1.0E-6 1.0E-7 1.0E-8 1.0E-9 1.0E-10 1.0E-11 1.0E-12 1.0E-13 1.0E-10

100cm 200cm 300cm 400 cm 500 cm

1.0E-8

1.0E-6

1.0E-4

Energy (GeV)

* Baseline parameters from Eurisol-DS #3 “100kW direct target station”

EURISOL Meeting, CEA Saclay, 27-28 October 2005

1.0E-2

1.0E+0

HIMAC benchmarck SELF-TOF detector configuration experiment arrangement

EURISOL Meeting, CEA Saclay, 27-28 October 2005

HIMAC benchmarck SELF-TOF detector configuration geometry model

EURISOL Meeting, CEA Saclay, 27-28 October 2005

HIMAC benchmarck SELF-TOF detector configuration Iron shielding -Preliminary results (1) 2

Comparison of measured and calculated neutron fluences (n sr-1 ion-1) Thickness (cm) Experiment 20 2.3290E+00

2

FLUKA 1.2516E+00

C/E 0.54

40

6.0284E-01

4.0127E-01

0.67

60

1.6060E-01

1.3848E-01

0.86

Attenuation length of the neutron fluence for SELF-TOF detector (cm) Experiment 123.

FLUKA 117.4

C/E 0.95 EURISOL Meeting, CEA Saclay, 27-28 October 2005

HIMAC benchmarck SELF-TOF detector configuration Iron shielding -Preliminary results (2) Comparison of measured and calculated neutron energy spectra SELF-TOF Iron 20cm

SELF-TOF Iron 60cm

SELF-TOF Iron 40cm

1.0E+0

1.0E+0

1.0E-2

1.0E-3

1.0E-4

Fluence (n/MeVsr//ion)

1.0E-1

Fluence (n/MeV/sr/ion)

Fluence (n/cm^2/sr/ion)

1.0E-1

Experiment

1.0E-3

FLUKA Experiment

FLUKA

1.0E-2 1.0E-3 1.0E-4 1.0E-5 1.0E-6

FLUKA Experiment

1.0E-4

1.0E-5

1.0E-7 1.0E-5

1.0E-6

1.0E-8 1.0E+1

1.0E+2

1.0E+3

1.0E+1

Enegy (M ev)

1.0E+2

SELF-TOF Iron 80cm

SELF-TOF Iron 100cm FLUKA

Fluence (n/MeV/sr/ion)

Exp e rime n t

Fluence (n/MeV/sr/ion)

1.0E+2

1.0E-3 FL U KA

1.0E-4

1.0E-5

1.0E-6

Experiment

1.0E-4

1.0E-5

1.0E-6

1.0E-7

1.0E-7 1.0E+1

1.0E+1

Energy (MeV)

Energy(Mev)

1.0E-3

2

1.0E+3

1.0E+2

Energy (MeV)

1.0E+3

1.0E+1

1.0E+2

1.0E+3

Energy (MeV)

EURISOL Meeting, CEA Saclay, 27-28 October 2005

1.0E+3

HIMAC benchmarck SELF-TOF detector configuration Concrete shielding -Preliminary results (1) 2

Comparison of measured and calculated neutron fluences (n sr-1 ion-1)

Thickness (cm) Experiment

2

FLUKA

C/E

50

2.526

1.371

0.543

100

0.655

0.453

0.691

Attenuation length of the neutron fluence for SELF-TOF detector (cm) Experiment 86.9

FLUKA 78.2

C/E 0.90

EURISOL Meeting, CEA Saclay, 27-28 October 2005

HIMAC benchmarck SELF-TOF detector configuration Concrete shielding -Preliminary results (2) Comparison of measured and calculated neutron energy spectra SELF-TOF concrete 50cm 1.0E-1

FLUKA

FLUKA Experiment

1.0E-2

1.0E-3

1.0E-4

Experiment

Fluence (n/MeV/sr/ion)

Fluence (n/MeV/sr/ion)

SELF-TOF concrete 100cm 1.0E-2

1.0E-3

1.0E-4

1.0E-5

1.0E-6

1.0E-5

1.0E-2

1.0E-2

1.0E-1

1.0E+0

1.0E-1

1.0E+0

Energy (MeV)

Energy (MeV)

SELF-STO concrete 200cm

SELF-TOF concrete 150cm

FLUKA Experiment

1.0E-3

1.0E-03

Fluence (n/MeV/sr/ion)

Experiment

1.0E-04

1.0E-05

1.0E-06

1.0E-07 1.0E-02

Fluence (n/MeN/sr/ion)

FLUKA

1.0E-4

1.0E-5

1.0E-6

1.0E-7

1.0E-8 1.0E-01

Energy (MeV)

1.0E+00

1.0E-2

1.0E-1

1.0E+0

Energy (MeV)

EURISOL Meeting, CEA Saclay, 27-28 October 2005

HIMAC benchmarck Discussions 1

1

Neutron spectra on the detector surface were obtained by surface current; Real model of the 12C on Cu target neutron source has been done by using RQMD-DPMJET FLUKA external event generator;

1

A FLUKA source subroutine of experimental secondary neutrons distribution has been created for comparison purposes;

1

Presented results are preliminary. Statistic should be improved;

1

Comparison of simulation results are in generally good agreement with experimental data.

1

Other two configurations of the HIMAC test problem: Ne213 detectors and Bi & C activation detectors have been modeled and calculations are in progress. EURISOL Meeting, CEA Saclay, 27-28 October 2005

Conclusions 1

1 1 1 1

Applicability of FLUKA Monte Carlo simulation in the design of biological shield of the high intensity neutron sources has been investigated; Basic shielding studies focused on the layout of the target station shield have been performed; Specific variance technique have been improved as a major part in the development of a design strategy ; Works are in progress to test the developed method by comparison with experimental data. A generally good agreement has been obtain; Technique developed can be easily extended to design studies of other installation components: accelerator, beam dump, etc

EURISOL Meeting, CEA Saclay, 27-28 October 2005